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Emission of Volatile Organic Compounds from the Residential Combustion of Pyrenean Oak and Black Poplar
Abstract:Smoke from domestic wood burning has been identified as a major contributor to air pollution, motivating detailed emission measurements under controlled conditions. A series of experiments was performed to characterise the emissions from wood combustion in a fireplace and in a woodstove of two common species of trees grown in Spain: Pyrenean oak (Quercus pyrenaica) and black poplar (Populus nigra). Volatile organic compounds (VOCs) in the exhaust emissions were collected in Tedlar bags, re-sampled in sorbent tubes and analysed by thermal desorption-gas chromatography-flame ionisation detection. Pyrenean oak presented substantially higher emissions in the woodstove than in the fireplace, for the majority of compounds. The opposite was observed for poplar. Among the 45 identified species, benzene and benzenerelated compounds represent the most abundant group, followed by oxygenated VOCs and aliphatics. Emission factors obtained in this study are generally of the same order than those reported for residential experiments in the USA.
Digital Object Identifier (DOI): doi.org/10.5281/zenodo.1061695Procedia APA BibTeX Chicago EndNote Harvard JSON MLA RIS XML ISO 690 PDF Downloads 1418
 C. Reche, M. Viana, F. Amato, Alastuey, T. Moreno, R. Hillamo, K. Teinil├ñ, K. Saarnio, R. Seco, J. Pe├▒uelas, C. Mohr, A.S.H. Prév├┤t, X. Querol, "Biomass burning contributions to urban aerosols in a coastal Mediterranean city", Sci. Total Environ., vol. 427-428, pp. 175-190, 2012.
 H. Puxbaum, A. Caseiro, A. Sanchez-Ochoa, A. Kasper-Giebl, M. Claeys, A. Gelencsér, M. Legrand, S. Preunkert, C. A. Pio, "Levoglucosan levels at background sites in Europe for assessing the impact of biomass combustion on the European aerosol background", J. Geophys. Res., vol. 112, D23S05, 2007.
 O. Favez, H. Cachier, J. Siare, R. Sarda-Estève, L. Martinon, "Evidence for a significant contribution of wood burning aerosols to PM2.5 during the winter season in Paris, France", Atmos. Environ., vol. 43, pp. 3640- 3644, 2009.
 A. Caseiro, H. Bauer, C. Schmidl, C.A. Pio, H. Puxbaum, "Wood burning impact on PM10 in three Austrian regions", Atmos. Environ., vol. 43, pp. 2186-2195, 2009.
 C. Gon├ºalves, C. Alves, M. Evtyugina, F. Mirante, C. Pio, A. Caseiro, C. Schmidl, H. Bauer, F. Carvalho, "Characterisation of PM10 emissions from wood stove combustion of common woods grown in Portugal", Atmos. Environ., vol. 44, pp. 4474-4480, 2010.
 C. Gon├ºalves, C. Alves C., A. P. Fernandes, C. Monteiro, L. Tarelho, M. Evtyugina, C. Pio, "Organic compounds in PM2.5 emitted from fireplace and woodstove combustion of typical Portuguese wood species", Atmos. Environ., vol. 45, pp. 4533-4545, 2011.
 C. Alves, C. Gon├ºalves, A. P. Fernandes, L. Tarelho, C. Pio, " Fireplace and woodstove fine particle emissions from combustion of western Mediterranean wood types", Atmos. Res., vol. 101, pp. 692-700, 2011.
 P. Ciccioli, E. Brancaleoni, M. Frattoni, A. Cecinato, L. Pinciarelli, "Determination of volatile organic compounds (VOC) emitted from biomass burning of Mediterranean vegetation species by GC-MS", Anal. Lett., vol. 34, pp. 937-955, 2001.
 A. K. Bolling, J. Pagels, K. E. Yttri, L. Barregard, G. Sallsten G., P. E., Schwarze, C. Boman, "Health effects of residential wood smoke particles: the importance of combustion conditions and physicochemical particle properties", Part. Fibre Toxicol., vol. 6:29, 2009.
 A. I. Calvo, L. A. C. Tarelho, M. Duarte, M. Evtyugina, C. A. Alves, "Operating conditions of a Portuguese wood stove" in Proc. 4th Int. Cong. Energ. Environ. Eng. Manage. (CIIEM), Merida, Spain, 2011.
 A. I. Calvo A.I., L.A.C. Tarelho, M. Duarte, T. Nunes, M. Evtyugina, C. Alves, C. Pio, A. Castro, R. Fraile, " A comparative study of particle emissions from Portuguese wood stove and fireplace devices" in Proc. Reuni├│n Espa├▒ola de Ciencia y Tecnolog├¡a de Aerosoles -RECTA. CIEMAT, Madrid, Spain, 2011.
 C. Boman, A. Nordin, R. Westerholm, E. Pettersson, "Evaluation of a constant volume sampling setup for residential biomass fired appliances - influence of dilution conditions on particulate and PAH emissions", Biomass Bioenerg., vol. 29, pp. 258-268, 2005.
 G. C. England, J. G. Watson, J. C. Chow, B. Zielinska, M. C. O. Chang, K. R. Loos, G. M. Hidy, "Dilution-based emissions sampling from stationary sources: part 1 - compact sampler methodology and performance", JAPCA J. Air Waste Ma., vol. 57, pp. 65-78, 2007.
 G. C. England, J. G. Watson, J. C. Chow, B. Zielinska, M. C. O. Chang, K. R. Loos, G. M. Hidy, "Dilution-based emissions sampling from stationary sources: part 2 - gas-fired combustors compared with other fuel-fired systems", JAPCA J. Air Waste Ma., vol. 57, pp. 79-93, 2007.
 P. M. Fine, G. R. Cass, B. R. T. Simoneit, "Chemical characterization of fine particle emissions from fireplace combustion of woods grown in the Midwestern and western United States", Environ. Eng. Sci., vol. 21, pp. 387-409, 2004.
 P. M. Fine, G. R. Cass, B. R. T. Simoneit, "Chemical characterization of fine particle emissions from the wood stove combustion of prevalent United States tree species", Environ. Eng. Sci., vol. 21, pp. 705-721, 2004.
 A. J. Scott. Real-life emissions from residential wood burning appliances in New Zealand. Ministry for the Environment. Christchurch, New Zealand, 65p, 2005.
 J. D. McDonald, B. Zielinska, E. M. Fujita, J. C. Sagebiel, J. C. Chow, J. G. Watson. "Fine Particle and Gaseous Emission Rates from Residential Wood Combustion", Environ. Sci. Technol., vol. 34, pp. 2080-2091, 2000.