Graphene/ZnO/Polymer Nanocomposite Thin Film for Separation of Oil-Water Mixture
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Graphene/ZnO/Polymer Nanocomposite Thin Film for Separation of Oil-Water Mixture

Authors: Suboohi Shervani, Jingjing Ling, Jiabin Liu, Tahir Husain

Abstract:

Offshore oil-spill has become the most emerging problem in the world. In the current paper, a graphene/ZnO/polymer nanocomposite thin film is coated on stainless steel mesh via layer by layer deposition method. The structural characterization of materials is determined by Scanning Electron Microscopy (SEM) and X-ray diffraction (XRD). The total petroleum hydrocarbons (TPHs) and separation efficiency have been measured via gas chromatography – flame ionization detector (GC-FID). TPHs are reduced to 2 ppm and separation efficiency of the nanocomposite coated mesh is reached ≥ 99% for the final sample. The nanocomposite coated mesh acts as a promising candidate for the separation of oil- water mixture.

Keywords: Oil-spill, graphene, oil-water separation, nanocomposite.

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[1] Carpenter A. “Oil pollution in the north sea: The impact of governance measures on oil pollution over several decades. Hydrobiologia, 845, 109-127, 2019.
[2] C. Safina, A Sea in Flames: The Deepwater Horizon Oil Blowout, US: Broadway paperbacks, Crown publishing group, 2011.
[3] R.Gramling and W. Freudenburg, Blowout in the Gulf: The BP Oil Spill Disaster and the Future of Energy in America. USA: MIT Press, 2011.
[4] T. Husain, Kuwaiti Oil Fires: Regional Environmental Perspectives. US:Pergamon press, Elsevier, 1995.
[5] P. Kajitvichyanukul, Y.-T. Hung and L. Wang, Handbook of Environmental Engineering, 4, 521, 2006.
[6] M. Cheryan and N. Rajagopalan, J. Membr. Sci., 151,13, 1998.
[7] J. Yang, Z. Zhang, X. Xu, X. Zhu, X. Men and X. Zhou. “Superhydrophilic–superoleophobic coatings”. Journal of Materials Chemistry,22, 2834–37, 2012.
[8] J. Li, L. Yan, W. Li, J. Li, F. Zha and Z. Lei, “Superhydrophilic underwater superoleophobic ZnO-based coated mesh for highly efficient oil and water separation”. Materials Letters, 153, 62–65, 2015.
[9] J. Li et al., “Superhydrophobic meshes that can repel hot water and strong corrosive liquids used for efficient gravity-driven oil/water separation”, Nanoscale, vol. 8, pp. 7638-7645, 2016.
[10] S. Li et al., “A review on special wettability textiles: theoretical models, fabrication technologies and multifunctional applications”, J. Mater. Chem. A, vol. 5, pp. 31–55, 2017.
[11] L. Zhang et al. “A self-cleaning underwater superoleophobic mesh for oil-water separation”, Sci. Rep., vol. 3, pp. 2326, 2013.
[12] J. Liu et al., “Synthesis of graphene oxide–SiO2 coated mesh film and its properties on oil–water separation and antibacterial activity”, Water Sci. Technol., vol. 73 no. 5, pp. 1098-103, 2016.
[13] Q. Wen et al., “Zeolite-coated mesh film for efficient oil–water separation”. Chem. Sci., vol. 4, pp. 591-595, 2013.
[14] J. Song et al. “Superhydrophilic cement coated mesh: An acid, alkali and organic reagent-free material for oil/water separation”, J Nanoscale, vol. 00, pp. 1-3, 2017.
[15] Y. Q. Liu et al. “Laser-structured Janus wire mesh for efficient oil-water separation”, Nanoscale, vol. 9, pp. 17933-17938, 2017.
[16] L. Xiong, W. Guo, B. M. Alameda, R. K. Sloan, W. D. Walker and D. L. Patton. Rational Design of Superhydrophilic/Superoleophobic Surfaces for Oil−Water Separation via Thiol−Acrylate Photopolymerization. ACS Omega, 3,10278−10285,2018.
[17] Qu M, Ma L., Zhou Y., Zhao Y,, Wang J., Zhang Y., Zhu X., Liu X. and He J., “Durable and Recyclable Superhydrophilic− Superoleophobic Materials for Efficient Oil/Water Separation and Water-Soluble Dyes Removal”. ACS Applied.Nano Materials, 1, 5197– 5209,2018
[18] Gao M. L., Zhao S. Y., Chen Z. Y., Liu L. and Han Z. B., “Superhydrophobic/Superoleophilic MOF Composites for Oil−Water Separation”. Inorganic Chemistry,.58,2261–2264,2019.
[19] Chen, J. et al. “An improved Hummers method for eco-friendly synthesis of graphene oxide”. Carbon, vol. 64, pp. 225-229, 2013.
[20] S. Shervani, et al. “Synthesis and structural evolution of ZnO/TiO2 nanocomposites”. AIP Conference Proceedings, vol. 277, pp. 1447, 2012.
[21] J-B Wu et al., “Raman spectroscopy of graphene-based materials and its applications in related devices”, Chem. Soc. Rev., vol. 47, pp. 1822, 2018
[22] Y Guo et al., “Intercalation Polymerization Approach for Preparing Graphene/Polymer Composites”, Polymers, vol. 10 no. 61, pp 1-28, 2018.
[23] K. A. Alim, et al. “Micro-Raman investigation of optical phonons in ZnO nanocrystals”, J. Appl. Phys., vol. 97, pp. 124313, 2005.