Distribution and Source of PAHs in Surface Sediments of Canon River Mouth, Taiwan
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Distribution and Source of PAHs in Surface Sediments of Canon River Mouth, Taiwan

Authors: Chiu-Wen Chen, Chih-Feng Chen, Cheng-Di Dong

Abstract:

Surface sediment samples were collected from the Canon River mouth, Taiwan and analyzed for polycyclic aromatic hydrocarbons (PAHs). Total PAHs concentrations varied from 337 to 1,252 ng/g dry weight, with a mean concentration of 827 ng/g dry weight. The spatial distribution of PAHs reveals that the PAHs concentration is relatively high in the river mouth region, and gradually diminishes toward the harbor region. Diagnostic ratios showed that the possible source of PAHs in the Canon River mouth could be petroleum combustion. The toxic equivalent concentrations (TEQcarc) of PAHs varied from 47 to 112 ng TEQ/g dry weight. Higher total TEQcarc values were found in the river mouth region. As compared with the US Sediment Quality Guidelines (SQGs), the observed levels of PAHs at Canon River mouth were lower than the effects range low (ERL), and would probably not exert adverse biological effects.

Keywords: PAHs, sediment, river mouth, sediment quality guidelines (SQGs), toxic equivalent (TEQcarc)

Digital Object Identifier (DOI): doi.org/10.5281/zenodo.1077016

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References:


[1] L.E. Sverdrup, T. Nielsen, and P.H. Krogh, "Soil ecotoxicity of polycyclic aromatic hydrocarbons in relation to soil sorption, lipophilicity, and water solubility," Environ. Sci. Technol., vol. 36, pp. 2429-2435, 2002.
[2] M. Qiao, C. Wang, S. Huang, D. Wang, and Z. Wang, "Composition, sources, and potential toxicological significance of PAHs in the surface sediments of the Meiliang Bay, Taihu Lake," China. Environ. Int., vol. 32, pp. 28-33, 2006.
[3] P.C. van Metre, B.J. Mahler, and E.T. Furlong, "Urban sprawl leaves its PAH signature," Environ. Sci. Technol., vol. 34, pp. 4064-4070, 2000.
[4] C.W. Chen, and C.F. Chen, "Distribution, Origin and Potential Toxicological Significance of Polycyclic Aromatic Hydrocarbons (PAHs) in Sediments of Kaohsiung Harbor, Taiwan," Mar. Pollut. Bull., vol. 63, pp. 417-423, 2011.
[5] P. Baumard, H. Budzinski, and P. Garrigues, "Polycyclic aromatic hydrocarbons (PAHs) in sediments and mussels of the western Mediterranean Sea," Environ. Toxicol. Chem., vol. 17, pp. 765-776, 1998.
[6] M.B. Yunker, R.W. Macdonald, R. Vingarzan, R.H. Mitchell, D. Goyette, and S. Sylvestre, "PAHs in the Fraser River Basin: a critical appraisal of PAH ratios as indicators of PAH source and composition," Org. Geochem., vol.33, pp. 489-515, 2002.
[7] H. Budzinski, I. Jones, J. Bellocq, C. Pierrad, and P. Garrigues, "Evaluation of sediment contamination by polycyclic aromatic hydrocarbons in the Gironde estuary," Mar. Chem., vol. 58, pp. 85-97, 1997.
[8] M.P. Zakaria, H. Takada, S. Tsutsumi, K. Ohno, J. Yamada, E. Kouno, and H. Kumata, "Distribution of polycyclic aromatic hydrocarbons (PAHs) in rivers and estuaries in Malaysia: a widespread input of petrogenic PAHs," Environ. Sci. Technol., vol.36, pp. 1907-1918, 2002.
[9] S.A. Stout, A.D. Uhler, and S.D. Emsbo-Mattingly, "Comparative evaluation of background anthropogenic hydrocarbons in surficial sediments from nine urban waterway," Environ. Sci. Technol., vol.38, pp. 2987-2994, 2004.
[10] G. De Luca, A. Furesi, G. Micera, A. Panzanelli, P.C. Piu, M.I. Pilo, N. Spano, and G. Sanna, "Nature, distribution and origin of polycyclic aromatic hydrocarbons (PAHs) in the sediments of Olbia Harbor (Northern Sardinia, Italy)," Mar. Pollut. Bull., vol.50, pp. 1223-1232, 2005.
[11] H.H. Soclo, P. Garrigues, and M. Ewald, "Origin of polycyclic aromatic hydrocarbons (PAHs) in coastal marine sediments: case studies in Cotonou (Benin) and Aquitaine (France) areas," Mar. Pollut. Bull., vol. 40, pp. 387-396, 2000.
[12] E. Magi, R. Bianco, C. Ianni, and M.D. Carro, "Distribution of polycyclic aromatic hydrocarbons in the sediments of the Adriatic Sea," Environ. Pollut., vol.119, pp. 91-98. , 2002.
[13] J. Zhang, L.Z. Cai, D.X. Yuan, and M. Chen, "Distribution and sources of polynuclear aromatic hydrocarbons in mangrove surficial sediments of Deep Bay, China," Mar. Pollut. Bull., vol.49, pp. 479-486, 2004.
[14] G. Li, X. Xia, Z. Yang, R. Wang, and N. Voulvoulis, "Distribution and sources of polycyclic aromatic hydrocarbons in the middle and lower reaches of the Yellow River," China. Environ. Pollut., vol. 144, pp. 985-993 , 2006.
[15] V.M. Savinov, T.N. Savinova, G.G. Matishov, S. Dahle, and K. Næc, "Polycyclic aromatic hydrocarbons (PAHs) and organochlorines (OCs) in bottom sediments of the Guba Pechenga, Barents Sea, Russia," Sci. Total Environ., vol.306, pp. 39-56, 2003.
[16] M. Nadal, M. Schuhmacher, and J.L. Domingo, "Levels of PAHs in soil and vegetation samples from Tarragona County, Spain," Environ. Pollut., vol.132, pp. 1-11, 2004.
[17] C.A. Peters, C.D. Knightes, and D.G.Brown, "Long-term composition dynamics of PAH-containing NAPLs and implications for risk assessment," Environ. Sci. Technol., vol.33, pp. 4499-4507, 1999.
[18] US EPA (US Environmental Protection Agency), "Provisional Guidance for Quantitative Risk Assessment of Polycyclic Aromatic Hydrocarbons," EPA/600/R/089, Washington, DC: office of research and development, 1993.
[19] E.R. Long, D.D. MacDonald, S.L. Smith, and F.D. Calder, "Incidence of adverse biological effects within ranges of chemical concentrations in marine and estuary sediments," Environ. Manage., vol. 19, pp. 81-97, 1995.