Decay Heat Contribution Analyses of Curium Isotopes in the Mixed Oxide Nuclear Fuel
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Decay Heat Contribution Analyses of Curium Isotopes in the Mixed Oxide Nuclear Fuel

Authors: S. S. Nafee, A. K. Al-Ramady, S. A. Shaheen

Abstract:

The mixed oxide nuclear fuel (MOX) of U and Pu contains several percent of fission products and minor actinides, such as neptunium, americium and curium. It is important to determine accurately the decay heat from Curium isotopes as they contribute significantly in the MOX fuel. This heat generation can cause samples to melt very quickly if excessive quantities of curium are present. In the present paper, we introduce a new approach that can predict the decay heat from curium isotopes. This work is a part of the project funded by King Abdulaziz City of Science and Technology (KASCT), Long-Term Comprehensive National Plan for Science, Technology and Innovations, and take place in King Abdulaziz University (KAU), Saudi Arabia. The approach is based on the numerical solution of coupled linear differential equations that describe decays and buildups of many nuclides to calculate the decay heat produced after shutdown. Results show the consistency and reliability of the approach applied.

Keywords: Decay heat, Mixed oxide nuclear fuel, Numerical Solution of Linear Differential Equations, and Curium isotopes

Digital Object Identifier (DOI): doi.org/10.5281/zenodo.1332758

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References:


[1] Tobias, Prog. Nucl. Energy, vol 5, 1982, pp. 1.
[2] IAEA 483, INDC(NDS)-0483, Summary Report of Consultants’ Meeting “Beta-decay and Decay Heat, IAEA Vienna, 12-14 December, 2005.
[3] IAEA 499, INDC(NDS)-0499, Summary Report of Second consultants’ Meeting “Beta-decay and Decay Heat, NEA Data Bank, Paris, May 3, 2006.
[4] F. Schmittroth, Nucl. Sci. Eng., vol 59, 1976, pp. 117.
[5] F.. Schmittroth and R. Schenter, Nucl. Sci. Eng., vol 63, 1977, pp. 276.
[6] H N. Haguara et. al., J. Nucl. Sci. and Technol., vol 43 2006, PP. 497.
[7] J. Katakura et. al., J. Nucl. Sci. and Technol., vol 38, 2001, PP. 470.
[8] J.A. Hardy et. al., Phys. Lett. B, vol 71, 1977, pp. 307.
[9] T. Yoshida et. al., J. Nucl. Sci. and Technol., vol 18, 1981, pp. 393.
[10] C.L. Duke et. al., Nucl. Phys. A, vol 151, 1970, pp. 609.
[11] R. Greenwood et. al., Nucl. Instr. and Meth., A, vol 390, 1997, pp. 95.
[12] O. Masahico, K. Shin-Chi, M. Katsufomi, N. Takashi and M. Toshiaki, J. Nucl. Sci. Tech., vol 38, 2001, pp. 912.
[13] Culbreth, E. Bakker and J. Vegatto, "The Fission Properties of Curium Separated from Spent Nuclear Fuel," UNLV report, Las Vegas, U.S.A., 2002.
[14] H. Bateman, Proc. Cambridge Philos. Soc. Vol 15, 1910, pp. 423
[15] Yuan, D. and Kernan,W., J. Appl. Phys., vol 101, 2007, pp. 094907.
[16] J. C. Butcher, "Numerical methods for ordinary differential equations," John Wiley & Sons, ISBN 0471967580, 2003.
[17] L. F. Shampine, "Numerical Solution of Ordinary Differential Equations,"
[18] L. F. Shampine, and M. W. Reichelt, Journal on Scientific Computing, vol 18, 1997, pp. 1.
[19] K. E. Brenan, S. L. Campbell, and L. R. Petzold, "Numerical Solution of Initial Value Problems in Differential-Algebraic Equations," SIAM, Philadelphia, 1996.
[20] P. Bogacki and L. F. Shampine, Applied Mathematics Letters, vol 2, 1989.